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As far as professions go, is it pretty much a tossup between alchemy (trinkets and mad alchemy potions), JC (trinkets and bop gems), engineering (goggles and rocket launcher for sta/pulling), and enchanting (ring enchants).
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Given how hard it can be to get a T5+ helm, engineering gives a huge boost. If you're in a guild that will regularly down Vashj/Arch, then I'd say sure - engineering isn't going to be stellar. Otherwise it's a huge win.
I personally think that eng/ench works best; engineering for a fairly hard-to-replace piece of gear, and enchanting for more spelldamage and a nice synergy with soloing instances.